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Multistage mass spectrometry and density functional theory (DFT) were used to characterise the small silver hydride nanocluster, [Ag3H2L]+ (where L=(Ph2P)2CH2) and its gas‐phase unimolecular chemistry. Collision‐induced dissociation (CID) yields [Ag2HL]+ as the major product while laser‐induced dissociation (LID) proceeds via H2 formation and subsequent release from [Ag3H2L]+, giving rise to [Ag3L]...
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