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Eins nach dem andern: Metallorganische Cyclopentadienyl‐IrIII‐Halbsandwichkomplexe mit N,N‐chelatbildenden Liganden können die Reduktion von Chinonen (Q) wie Vitamin K3 zu Semichinonen (Q.−) durch Coenzym NADH katalysieren (siehe Bild). DFT‐Rechnungen sprechen für einen Mechanismus, der einen Hydridtransfer mit zwei nachfolgenden Einelektronentransfers sowie den unüblichen IrII‐Oxidationszustand im...
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