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The good co‐existence of midgap state and valence band degeneracy is realized in Bi‐alloyed GeTe through the In‐Cd codoping to play different but complementary roles in the valence band structure modification. In doping induces midgap state and results in a considerably improved Seebeck coefficient near room temperature, while Cd doping significantly increases the Seebeck coefficient in the mid‐high...
The emerged strategy of entropy engineering provides new ideas for realizing high‐performance thermoelectric materials, but it is still much unresolved how to achieve delicate trade‐off between the carrier mobility mH and the lattice thermal conductivity κph in taking advantage of configurational entropy ΔS. Herein, the significant advances of ultralow κph yet decent mH in a new medium‐entropy system...
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