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Designer SMM: An ErIII‐based single‐molecule magnet (SMM) was synthesized by designing the ligand‐field anisotropy around an ErIII ion in an equatorial arrangement of donors using a rigid and planar macrocyclic Schiff base ligand including three ZnII ions. The resulting ErIIIZnII3 complex (see picture; C gray, O red, N blue) behaves as a SMM with an energy barrier of 24.6(9) K for flipping of the...
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