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The synthesis, molecular structure as well as in situ spectroelectrochemical and electron spin resonance (ESR) studies of 5,7,8,10,15,17,18,20-octaphenyl-21,23-dithiaporphyrin (S2OPP) are presented. The compound investigated can be reversibly oxidised and reduced to yield the corresponding stable monocation and monoanion species, respectively. The experimental ESR spectrum of S2OPP•+ can be simulated...
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