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Sum‐frequency spectroscopy (SFS) was used in an attempt to detect the platinum–carbon vibration of CO adsorbed on Pt(111). The international free‐electron laser FELIX at the FOM Institute, Rijnhuizen, provided the required tunable far‐infrared (19–23 µm) source, while complementary measurements in the C–O stretch region (4.7–5.1 µm) were performed at the University of Oxford with a conventional nanosecond...
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