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We present a new methodology to predict the enantioselectivity of asymmetric catalysis based on quantitative quadrant‐diagram representations of the catalysts and quantitative structure–selectivity relationship (QSSR) modelling. To account for quadrant occupation, we used two types of molecular steric descriptors: the Taft–Charton steric parameter (ν(Charton)) and the distance‐weighted volume (VW)...
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