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Zintl phases are renowned for their diverse crystal structures with rich structural chemistry and have recently exhibited some remarkable heat‐ and charge‐transport properties. The ternary bismuthides RELi3Bi2 (RE = La–Nd, Sm, Gd, and Tb) (namely, lanthanum trilithium dibismuthide, LaLi3Bi2, cerium trilithium dibismuthide, CeLi3Bi2, praseodymium trilithium dibismuthide, PrLi3Bi2, neodymium trilithium...
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