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Amphiphilic triblock copolymers containing FeIII‐catecholate complexes formulated as spherical‐ or cylindrical‐shaped micellar nanoparticles (SMN and CMN, respectively) are described as new T1‐weighted agents with high relaxivity, low cytotoxicity, and long‐term stability in biological fluids. Relaxivities of both SMN and CMN exceed those of established gadolinium chelates across a wide range of...
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