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For the development of all‐solid‐state lithium metal batteries (LMBs), a high‐porous silica aerogel (SA)‐reinforced single‐Li+ conducting nanocomposite polymer electrolyte (NPE) is prepared via two‐step selective functionalization. The mesoporous SA is introduced as a mechanical framework for NPE as well as a channel for fast lithium cation migration. Two types of monomers containing weak‐binding...
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