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NO x storage and NO oxidation experiments have been carried out on a model Pt/BaO/Al 2 O 3 catalyst powder in order to elucidate kinetic and thermodynamic limitations. Uptake of NO on a pre-oxidized catalyst reveals the existence of multiple regimes. The short-term storage is a sensitive function of storage time, but is nearly independent of temperature whereas the long-time...
The performance of a Pt/BaO/Al 2 O 3 washcoated monolith reactor is investigated using propylene as a reductant. The dependence of the time-averaged NO X conversion is reported for several operating parameters, including feed composition, temperature, flow rate, propylene pulse duration and overall cycle time. NO X storage data, which reveal both kinetic and thermodynamic...
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