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It is still poorly understood how the first intermediates of CO2 reduction are formed and converted to multi‐carbon products over Cu‐based electrodes. Herein, Ag is used to decorate dendritic Cu and a high Faradaic efficiency (FE) for C2H4 (25 %) is obtained on a CuAg electrode, which is about five times higher than dendritic Cu. The intermediates including *CO2−, OH groups, Cu‐CO, C‐O rotation, and...
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