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Femtochemie. In ihrer Zuschrift auf S. 10758 ff. berichten E. T. J. Nibbering, T. Elsaesser et al. über ultraschnelle Pump‐Probe‐Infrarotspektroskopie am Zundel‐Kation.
The nature of the excess proton in liquid water has remained elusive after decades of extensive research. In view of ultrafast structural fluctuations of bulk water scrambling the structural motifs of excess protons in water, we selectively probe prototypical protonated water solvates in acetonitrile on the femtosecond time scale. Focusing on the Zundel cation H5O2+ prepared in room‐temperature acetonitrile,...
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