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In article number 2004744, Zhendong Fu, Yan‐Zhen Zheng, and co‐workers report a van der Waals 2D magnetic material bearing a spin‐integer dimerized honeycomb lattice. This material can be prepared down to ten layers (13 nm in thickness) and exhibits a reentrant spin glass behavior with very hard magnetic hysteresis. Owing to the dedicated chemical design, this work successfully combines topological...
2D magnetic materials with dimerized honeycomb lattices can be treated as mixed‐spin square lattices, in which a quantum phase transition may occur to realize the Bose–Einstein condensation of magnons under reachable experimental conditions. However, this has never been successfully realized with integer spin centers. Herein, a spin integer (S = 2) dimerized honeycomb lattice in an iron(II)‐azido...
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