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In this work we demonstrate how hydrogen can be utilized to fine tune the emission gap of C60 through the formation of direct CH bonds in sodium and lithium intercalated systems (M6C60Hx). Upon hydrogenation, a shift in the emission spectrum to shorter wavelengths (higher energy) is observed relative to alkali metal free fulleranes (C60Hx) and pure C60. This is attributed to the higher degree of hydrogenation...
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