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Tetravalent tellurium ion conduction in solids has been demonstrated in α‐Te2MoO7 by both experimental and theoretical means for the first time. Although it has been commonly considered that the Te4+ ion will not conduct appreciably in solids due to its high valency, such conduction can be successfully achieved in solid α‐Te2MoO7, which has a 2D layered structure conducive to ion migration. The measured...
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