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Azobenzene‐containing crosslinked ferroelectric liquid‐crystalline polymers offer unique opportunities for reversible, high‐contrast switching of a second‐order nonlinear optical response in the solid state. Atsushi Shishido and co‐workers show on p. 6410 that this is achieved by reversibly controlling non‐centrosymmetric chromophore alignment through two‐photon isomerization of azobenzene molecules...
A conceptually novel materials design, based on crosslinked ferroelectric liquid‐crystalline polymers, is demonstrated for efficient switching of a second‐order nonlinear optical (NLO) response in the solid state. By controlling the molecular alignment of the NLO moieties through two‐photon isomerization of azobenzene molecules, reversible isothermal photocontrol of second‐harmonic generation is achieved...
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