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Ni‐Co layered double hydroxides (LDH) have received considerable attention as excellent pseudocapacitor electrode materials. In this paper, a novel utilization of the composite of graphene oxide (GO) and single‐walled carbon nanohorns (SWCNHs) is reported as an effective substrate for LDH coatings. We successfully synthesized hierarchical nanostructures composed of Ni‐Co LDH as well as microsphere...