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Cyclic organic ammoniums have been regarded as the suitable organic components for constructing the organic–inorganic hybrid phase transition materials because they have flexible cyclic structure. Here, an In‐based organic–inorganic hybrid compound, [C3H8N]3InBr6 (1; C3H8N+ is cyclopropylammonium), has been successfully synthesized. It is noteworthy that 1 experiences an invertible phase transition...
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