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A metal-organic framework, UiO-66, has been evaluated as adsorbent in a post-combustion vacuum swing adsorption (VSA) process. Equilibrium isotherms of the most relevant gases (CO2 and N2) as well as breakthrough curves measured using synthetic flue gas containing 15 mol% CO2 without and with 9 mol% water vapor are reported. Based on the breakthrough data, a six step one-column VSA cycle is designed...
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