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The concerted redox action of a metal ion and an organic cofactor is a unique way to maximize the catalytic power of an enzyme. An example of such synergy is the fungal galactose 6‐oxidase, which has inspired the creation of biomimetic copper oxidation catalysts. Galactose 6‐oxidase and its bacterial homologue, GlxA, possess a metalloradical catalytic site that contains a free radical on a covalently...
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