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Synthetic helical peptides are valuable scaffolds for the development of modulators of protein–protein interactions involving helical motifs. Backbone‐to‐side chain or side chain‐to‐side chain constraints have been and still are intensively exploited to stabilize short α‐helices. Very often, these constraints have been combined with backbone modifications induced by Cα‐tetrasubstituted, β‐, or γ‐amino...
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