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Fluorobenzene probes for protein profiling through selective cysteine labeling have been developed by rational reactivity tuning. Tuning was achieved by selecting an electron‐withdrawing para substituent in combination with variation of the number of fluorine substituents. Optimized probes chemoselectively arylated cysteine residues in proteins under aqueous conditions. Probes linked to azide, biotin,...
Ortsselektive Cystein‐Arylierung wurde durch rationale Reaktivitätsfeinabstimmung von Fluorbenzolsonden erreicht. M. Meldal, F. Diness et al. demonstrieren in ihrer Zuschrift auf S. 8154 ff., wie die Sonden auf die selektive Erkennung von Cystein‐haltigen Proteinen abgestimmt werden können, nämlich über die Zahl der Fluorsubstituenten (Fx) und durch die gezielte Auswahl der Substituenten basierend...
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