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Manganese(IV)‐oxo complexes are often invoked as intermediates in Mn‐catalyzed C−H bond activation reactions. While many synthetic MnIV‐oxo species are mild oxidants, other members of this class can attack strong C−H bonds. The basis for these reactivity differences is not well understood. Here we describe a series of MnIV‐oxo complexes with N5 pentadentate ligands that modulate the equatorial ligand...
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