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A series of platinum(II) diimine complexes with different substituents on fluorenyl acetylide ligands (1 a–1 e) were synthesized and characterized. The influence of the auxiliary substituent on the photophysics of these complexes has been systematically investigated spectroscopically and theoretically (using density functional theory (DFT) methods). All complexes exhibit ligand‐centered 1π,π* transitions...
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