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In article number 1808300, Daisuke Yokoyama, Hisahiro Sasabe, Junji Kido, and co‐workers demonstrate control over the molecular aggregation state in organic semiconductor films during vapor deposition. Synergetic effects of disordered hydrogen bonds and planar anisotropic molecular shapes enhance the horizontal molecular orientation and significantly increase the electron mobility. Moreover, the molecular...
Use of the intrinsic optoelectronic functions of organic semiconductor films has not yet reached its full potential, mainly because of the primitive methodology used to control the molecular aggregation state in amorphous films during vapor deposition. Here, a universal molecular engineering methodology is presented to control molecular orientation; this methodology strategically uses noncovalent,...
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