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Ab initio calculations of the two title reactions have been made to compare reactivities of OCS and CS 2 toward a nucleophile, NH2-. MP2/6-311++G(d, p) geometry optimizations on the singlet potential energy surface have demonstrated that respective channels start from key intermediates and have revealed that multistep paths give the most favorable products: (1) NH2-+OCS→H 2 NS ...
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