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The role of the interface between an MoOx anode interlayer and a polymer:fullerene bulk heterojunction is investigated. Processing differences in the MoOx induce large variations in the vertical stratification of the bulk heterojunction films. These variations are found to be inconsistent in predicting device performance, with a much better gauge being the quantity of polymer chemisorbed to the anode...
The interfacial microstructure in organic bulk heterojunction solar cells can dictate photovoltaic performance. By controlling the chemical interactions of bulk heterojunction components with specific surfaces, the electrical pathways at interfaces can be precisely varied to achieve suitable electronic properties across such interfaces. This is studied by J. J. Jasieniak and co‐workers on page 3944...
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