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We investigate the electronic decay of an Ar 3s-1 vacancy in medium sized ArKr clusters. The only energetically accessible, radiationless decay mechanism is Electron Transfer Mediated Decay Three (ETMD3). Here, the argon vacancy is filled by an electron from one krypton atom, and the excess energy is transferred to a second krypton atom which consequently emits an electron. For the theoretical calculation...
In this work we discuss the theoretical photo-double ionization spectrum of iodomethane which was obtained by the newly developed relativistic two-particle propagator and compare it to experimental data. For a correct interpretation of the spectral features in the outer valence region, spin–orbit effects play a major role and induce new features to the spectra. Additionally, wide-energy range single...
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