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The rate coefficient for the vibrational relaxation of isotopically-pure 13CO2 by ground state oxygen atoms was measured between 239 and 358K. O3 was photolyzed in a slow-flowing mixture of 13CO2, O3, and Xe to simultaneously create O atoms and stimulate a temperature-jump, shifting population into the first vibrationally-excited state of 13CO2. The population redistribution was monitored via transient...
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