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LF‐Muon Spin Relaxation data are reported for the organometallic compounds Pb(C6H5)4, (C6H6)Cr(CO)3 and (C5H5)2Ru. In each case the change in relaxation rate with temperature shows a peak analogous to the T_1 minimum in NMR. The activation parameters were calculated, and the mechanism of muon spin relaxation in the case of (C6H6)Cr(CO)3 is shown to be the reorientation motion of the benzene ring.
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