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Magnetic‐energy harvesting in a centimeter‐sized free‐standing (BEDT‐TTF)C60 charge‐transfer single crystal is demonstrated. The crystal shows sensitive magnetic‐, thermal‐, and mechanical‐sensing ability, with an excellent piezoresistance coefficient of −5.1 × 10−6 Pa−1. The self‐powered sensing performance, together with its solution processability and flexibility, endow it with the capability of...