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Femtosecond pump probe spectroscopy was employed to measure intramolecular vibrational energy redistribution (IVR) and intermolecular vibrational energy transfer (VET) of benzene in the gas phase and in supercritical (sc) CO 2 . We observe two IVR time scales the faster of which proceeds within τIVR(1)<0.5ps. The slower IVR component has a time constant of τIVR(2)=(48±5)ps in the gas phase...
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