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Die Verteilung von Ladungen innerhalb pH‐responsiver Wirkstoffträger beeinflusst nachweislich die Effizienz der Freisetzung, ist aber schwer zu kontrollieren und zu verifizieren. Wir stellen nun polyampholytische Nanogel‐in‐Mikrogel Kolloide (NiM−C) vor und zeigen, dass die Anordnung der Nanogele (NG) abhängig von den Synthesebedingungen ist. Dazu wurden pH‐responsive Polyelektrolyt‐NG durch Fällungspolymerisation...