Two manganese(III)‐dicyanamide compounds, [Mn(5‐Brsalen)(dca)]·CH3OH (1) and [Mn(3‐Meosalphen)(dca)(H2O)] (2) (dca = dicyanamide anion, [N(CN)2]–), were synthesized and characterized by elemental analysis, IR spectroscopy, single‐crystal X‐ray structure analysis, and cyclic voltammetry. The structure of complex 1 is an infinite zigzag chain of hexacoordinate MnIII ions, in which the adjacent manganese...
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