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KCrS2 is presented as a stable and high‐rate layered material that can be used as a cathode in potassium‐ion batteries. As far as it is known, KCrS2 is the only layered material with stoichiometric amounts of K+, which enables coupling with a graphite anode for full‐cell construction. Cr(III)/Cr(IV) redox in KCrS2 is also unique, because LiCrS2 and NaCrS2 are known to experience S2−/S22− redox. O3‐KCrS...
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