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Inspired by the hierarchically helical structure of classical thermal insulation material—wool, a stretchable heating carbon nanotube (CNT) fiber is created with excellent mechanical and heating properties. It can be stretched by up to 150% with high stability and reversibility, and a good thermal insulation is achieved from a large amount of formed hierarchically helical voids inside. Impressively,...
The equimolar C2H2‐CO2 reaction has shown promise for carbon nanotube (CNT) production at low temperatures and on diverse functional substrate materials; however, the electron‐pushing mechanism of this reaction is not well demonstrated. Here, the role of CO2 is explored experimentally and theoretically. In particular, 13C labeling of CO2 demonstrates that CO2 is not an important C source in CNT growth...
Direct growth of chirality‐controlled single‐walled carbon nanotubes (SWNTs) with metal catalyst free strategy, like cloning or epitaxial growth, has suffered from the low efficiency. The underlying problem is the activation of seed edge. Here an unexpectedly efficient microwave‐assisted pathway to regenerate SWNTs from carbon fragments on SiO2/Si substrate is demonstrated via Raman spectroscopy and...
Inspired by the epidermal–dermal and outer microstructures of the human fingerprint, a novel flexible sensor device is designed to improve haptic perception and surface texture recognition, which is consisted of single‐walled carbon nanotubes, polyethylene, and polydimethylsiloxane with interlocked and outer micropyramid arrays. The sensor shows high pressure sensitivity (−3.26 kPa−1 in the pressure...
Distinguishable detection of the ultraviolet, visible, and infrared spectrum is promising and significant for the super visual system of artificial intelligences. However, it is challenging to provide a photosensor with such broad spectral response ability. In this work, the ultraviolet, visible, and infrared spectrum is distinguished by developing serial photosensors based on perovskite/carbon nanotube...
The high aspect ratio and the porous nature of spatially oriented forest‐like carbon nanotube (CNT) structures represent a unique opportunity to engineer a novel class of nanoscale assemblies. By combining CNTs and conformal coatings, a 3D lightweight scaffold with tailored behavior can be achieved. The effect of nanoscale coatings, aluminum oxide (Al2O3) and nonstoichiometric amorphous silicon carbide...
Carbon nanotubes (CNTs) interlocked by cyclic compounds through supramolecular interaction are promising rotaxane‐like materials applicable as 2D and 3D networks of nanowires and disease‐specific theranostic agents having multifunctionalities. Supramolecular complexation of CNTs with cyclic compounds in a “ring toss'' manner is a straightforward method to prepare interlocked CNTs; however, to date,...
In article number 1800720, Koji Miki, Kouichi Ohe, and co‐workers report the “ring toss” method, throwing carbon nanorings onto carbon nanotubes, to prepare “tube‐in‐ring” supramolecular complexes. Carbon nanorings, [n]cycloparaphenyleneacetylenes, are utilized to demonstrate the formation of “tube‐in‐ring” complexes. The good size fit between the concave inner surface of the carbon nanorings and...
Fiber‐shaped supercapacitors with improved specific capacitance and high rate capability are a promising candidate as power supply for smart textiles. However, the synergistic interaction between conductive filaments and active nanomaterials remains a crucial challenge, especially when hydrothermal or electrochemical deposition is used to produce a core (fiber)–shell (active materials) fibrous structure...
Compactness and versatility of fiber‐based micro‐supercapacitors (FMSCs) make them promising for emerging wearable electronic devices as energy storage solutions. But, increasing the energy storage capacity of microscale fiber electrodes, while retaining their high power density, remains a significant challenge. Here, this issue is addressed by incorporating ultrahigh mass loading of ruthenium oxide...
For the efficient recognition and classification of numerous images, neuroinspired deep learning algorithms have demonstrated their substantial performance. Nevertheless, current deep learning algorithms that are performed on von Neumann machines face significant limitations due to their inherent inefficient energy consumption. Thus, alternative approaches (i.e., neuromorphic systems) are expected...
The ingenious design of a freestanding flexible electrode brings the possibility for power sources in emerging wearable electronic devices. Here, reduced graphene oxide (rGO) wraps carbon nanotubes (CNTs) and rGO tightly surrounded by MnO2 nanosheets, forming a 3D multilevel porous conductive structure via vacuum freeze‐drying. The sandwich‐like architecture possesses multiple functions as a flexible...
In article number 1802225, Joselito M. Razal and co‐workers fabricate MXene‐based yarn‐shaped supercapacitors via biscrolling, which show ultrahigh MXene loading, excellent flexibility, and superior energy storage performance. The biscrolled MXene yarns with outstanding specific capacitance and energy density can potentially provide the energy solution for powering wearable electronics.
Yarn‐shaped supercapacitors (YSCs) once integrated into fabrics provide promising energy storage solutions to the increasing demand of wearable and portable electronics. In such device format, however, it is a challenge to achieve outstanding electrochemical performance without compromising flexibility. Here, MXene‐based YSCs that exhibit both flexibility and superior energy storage performance by...
Flexible transparent conductors are an enabling component for large‐area flexible displays, wearable electronics, and implantable medical sensors that can wrap around and move with the body. However, conventional conductive materials decay quickly under tensile strain, posing a significant hurdle for functional flexible devices. Here, we show that high electrical conductivity, mechanical stretchability,...
Carbon nanotube metals in a polydimethylsiloxane composite exhibit distinct electromechanical responses under high tensile strain. In article number 1802625, YuHuang Wang and co‐workers demonstrate that long nanotubes efficiently bridge strain‐induced cracks in the composite, maintaining high conductivity even after 1000 stretch‐release cycles, while short nanotubes respond sensitively to shape changes,...
Flexible supercapacitors have shown enormous potential for portable electronic devices. Herein, hierarchical 3D all‐carbon electrode materials are prepared by assembling N‐doped graphene quantum dots (N‐GQDs) on carbonized MOF materials (cZIF‐8) interweaved with carbon nanotubes (CNTs) for flexible all‐solid‐state supercapacitors. In this ternary electrode, cZIF‐8 provides a large accessible surface...
In article number 1702145, In‐Suk Choi, Youngjin Jeong, Ji‐Hoon Lee, and co‐workers design a new type of mechanically robust electrochemical capacitor for wearable electronics based on all‐carbon‐based self‐supported nanocomposites. By optimizing the architecture of the three‐dimensional nanocomposite structure with activated carbons uniformly embedded in carbon nanotube sheets, outstanding durability...
With the growing demand for wearable electronics, developing new compatible energy systems is a prominent topic of research. Energy systems mounted on wearable electronics should exhibit high cost efficiency, mechanical robustness, and high electrochemical activity. Herein, all‐carbon‐based large‐area nanocomposites for freely deformable electrochemical capacitors are suggested to address these requirements...
Efficient utilization of abundant solar energy for clean water generation is considered a sustainable and environment friendly approach to mitigate the global water crisis. For this purpose, this study reports a flexible fire‐resistant photothermal paper by combining carbon nanotubes (CNTs) and fire‐resistant inorganic paper based on ultralong hydroxyapatite nanowires (HNs) for efficient solar energy‐driven...
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