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The synthesis of the germacalicene 7 from the reaction of the dipotassium germole dianion K2[6] with 1,2‐bis‐diisopropylamino‐3‐chlorocyclopropenyl perchlorate is reported. Based on the crystal structure analysis and the results of DFT calculations, the germacalicene 7 can be viewed as a cyclopropenium germacyclopentadienide ylide that is isoelectronic to α‐cationic phosphanes. First reactivity studies...
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