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Der Quantentunneleffekt in einem einkernigen Dysprosium‐Einzelmolekülmagnet (SMM) lässt sich stark reduzieren, was dessen Speicherfähigkeit für magnetische Information verbessert. O. Cador und Mitarbeiter gelingt dies in ihrer Zuschrift auf S. 1524 ff. durch den Einsatz von DyIII‐Isotopen ohne kernmagnetisches Moment und durch Verdünnen des SMM in einer diamagnetischen Matrix. Diese Strategie öffnet...
The influence of nuclear spin on the magnetic hysteresis of a single‐molecule is evidenced. Isotopically enriched DyIII complexes are synthesized and an isotopic dependence of their magnetic relaxation is observed. This approach is coupled with tuning of the molecular environment through dilution in an amorphous or an isomorphous diamagnetic matrix. The combination of these approaches leads to a dramatic...
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