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We report the F2@C60 system as the first example of an endohedral fullerene in which C60 acts as a cation C60+ interacting with endohedral anion, F2−. Our state‐of‐the‐art computations reveal that in F2@C60, despite of the known high electron affinity of C60, an electron is transferred from C60 to F2 resulting in the F2−@C60+ system. The F−F bond length in F2@C60 is substantially longer than in free...
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