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The CuO+ core is a central motif of reactive intermediates in copper‐catalysed oxidations occurring in nature. The high reactivity of CuO+ stems from a weak bonding between the atoms, which cannot be described by a simple classical model. To obtain the correct picture, we have investigated the acetonitrile‐ligated CuO+ ion using neon‐tagging photodissociation spectroscopy at 5 K. The spectra feature...
Die Gegenwart einer [CuO]+‐Einheit wurde oft herangezogen, um die einzigartige Oxidationsreaktivität Cu‐haltiger Enzyme zu erklären. M. Srnec, J. Roithová et al. schildern in ihrer Zuschrift auf S. 17299 ff. die Nutzung kryogener Spektroskopie von gasförmigem, ligiertem CuO+, um die ersten hoch aufgelösten spektroskopischen Daten für diese Komplexe zu erhalten und so ein Licht auf die Cu‐O‐Bindung...
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