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Hierarchical porosity and functionalization help to fully make use of metal–organic frameworks (MOFs) for their diverse applications. Herein, a simple strategy is reported to construct hierarchically porous MOFs through a competitive coordination method using tetrafluoroborate (M(BF4)x, where M is metal site) as both functional sites and etching agents. The resulting MOFs have in situ formed defect‐mesopores...
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