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The experimental crystal structure and corresponding theoretical electron density determination of 2-hydroxy-4,4-dimethyl-6-oxo-cyclohex-1-ene carboxy amide is reported with special focus on two adjacent intramolecular hydrogen bonds (O–H⋯O and N–H⋯O). The possible tautomeric forms are studied and their theoretical populations in the gas phase were determined. Additionally, theoretical models which...
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