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Femtosecond-resolved broadband fluorescence studies are reported for[M(bpy) 3 ] 2+ (M=Fe, Ru), RuN3 and RuN719 complexes in solution. We investigated the pump wavelength dependence of the fluorescence of aqueous [Fe(bpy) 3 ] 2+ and the solvent and ligand dependence of the fluorescence of Ru-complexes excited at 400nm. For all complexes, the 1 MLCT fluorescence...
Fluorescence excitation spectra and fluorescence lifetimes at single vibronic levels in the S1 state have been observed for jet-cooled pyrene. The fluorescence lifetimes at the zero-vibrational levels of the S11B3u states of pyrene-h10 and pyrene-d10 are 1480 and 1470ns, respectively, and the relaxation is considered to be dominated by the radiative process. For some vibrational levels, however, the...
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