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A highly practical metal-free catalytic system has been developed for aerobic oxidation of alcohols to corresponding ketones and aldehydes using catalytic amount of N-hydroxyphthalimide (NHPI) and tert-butyl nitrite (TBN) with molecular oxygen serving as the terminal oxidant. A variety of aliphatic, aromatic, allylic, and heterocyclic alcohols were smoothly converted to desired products with moderate...
A series of isolated or preformed in-situ aliphatic PNP-type pincer ruthenium complexes have been evaluated for deuterium labelling of alcohols' C-H functions with deuterium oxide. Under our catalytic conditions, pincer-supported ruthenium complexes bearing cyclohexyl substituents on the phosphorous atoms have been found to be the most efficient and regioselective catalysts for α-deuteration of primary...
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