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The local structure and molecular motion for 133Cs in a Cs2CoBr4 single crystal were examined by using the spin-lattice relaxation time from nuclear magnetic resonance (NMR). The two inequivalent Cs(1) and Cs(2) sites surrounded by Br ions in Cs2CoBr4 were clearly distinguished by using 133Cs NMR spectra. The spin-lattice relaxation times T1 of the Cs(1) and Cs(2) nuclei in Cs2CoBr4 were obtained,...
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