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  • For some selected reviews in organocatalysis, see: a) Berkessel A., Göger H., Asymmetric Organocatalysis, WILEY-VCH, Weinheim, Germany, 2005. b) Dalko P. I., Enantioselective Organocatalysis, WILEY-VCH, Weinheim, 2007. c) Dalko P. I., Enantioselective Organocatalysis, Wiley- VCH, Weinheim, 2007. d) MacMillan D. W. C., The Advent and Development of Organocatalysis, Nature, 2008, 455, 304-308. e) Moyano A., Rios R., Asymmetric Organocatalytic Cyclization and Cycloaddition Reactions, Chem. Rev. 2011, 111, 4703-4832. f) Bernardi L., Fochi M., Franchini M. C., Ricci A., Bioinspired Organocatalytic Asymmetric Reactions, Org. Biomol. Chem. 2012, 10, 2911-2922. g) Cabrera S., Alemán J., Applications of Asymmetric Organocatalysis in Medicinal Chemistry, Chem. Soc. Rev. 2013, 42, 774-793.

  • For a seminal work in HOMO activation via enamine intermediates, see: a) List B., Lerner R. A., Barbas III C. F. J., Proline-Catalyzed Direct Asymmetric Aldol Reactions, J. Am. Chem. Soc., 2000, 122, 2395-2396. For a review in enamine activation, see: b) Mukherjee S., Yang J. W., Hoffmann S., List B., Asymmetric Enamine Catalysis, Chem. Rev. 2007, 107, 5471-5569. For a seminal work in HOMO-activation via dienamine intermediates, see: c) Bertelsen S., Marigo M., Brandes S., Dinér P., Jørgensen K. A., Dienamine Catalysis: Organocatalytic Asymmetric γ-Amination of α,β-Unsaturated Aldehydes, J. Am. Chem. Soc. 2006, 128, 12973-12980. For reviews in dienamine activation, see: d) Ramachary D. B., Reddy Y. V., Dienamine Catalysis: An Emerging Technology in Organic Synthesis, Eur. J. Org. Chem., 2012, 865-887. e) Parra A., Reboredo S., Alemán J., Asymmetric Synthesis of Cyclobutanes by a Formal [2+2] Cycloaddition Controlled by Dienamine Catalysis, Angew. Chem. Int. Ed. 2012, 51, 9734- 9735.

  • For a seminal work in LUMO activation, see: a) Ahrendt K. A., Borths C. J., MacMillan D. W. C., New Strategies for Organic Catalysis: The First Highly Enantioselective Organocatalytic Diels−Alder Reaction, J. Am. Chem. Soc. 2000, 122, 4243- 4244. For a review in LUMO activation, see: b) Erkkilä A., Majander I., Pihko P. M., Iminium Catalysis, Chem. Rev. 2007, 107, 5416-5470.

  • For a seminal work in SOMO activation, see: a) Beeson T. D., Mastracchio A., Hong J., Ashton K., MacMillan D. W. C., Enantioselective Organocatalysis Using SOMO Activation, Science 2007, 316, 582-585. For selected examples, see: b) Kim H., MacMillan D. W. C., Enantioselective Organo- SOMO Catalysis: The α-Vinylation of Aldehydes, J. Am. Chem. Soc. 2008, 130, 398-399. c) Rendler S., MacMillan D. W. C., Enantioselective Polyene Cyclization via Organo- SOMO Catalysis, J. Am. Chem. Soc. 2010, 132, 5027-5029. d) Jui N.T., Lee E. C., MacMillan D. W. C., Enantioselective Organo-SOMO Cascade Cycloadditions: A Rapid Approach to Molecular Complexity from Simple Aldehydes and Olefins, J. Am. Chem. Soc. 2010, 132, 10015-10017. e) Devery J J., Conrad J. C., MacMillan D. W. C., Flowers R. A., Mechanistic Complexity in Organo–SOMO Activation, Angew. Chem., Int. Ed. 2010, 49, 6106-6110.

  • For a review, see: a) Mikami K., Shimizu M., Zhang H.–C., Maryanoff B. E., Acyclic Stereocontrol between Remote Atom Centers via Intramolecular and Intermolecular Stereocommunication, Tetrahedron 2001, 57, 2917-2951. For selected examples, see: b) Linnane P., Magnus N., Magnus P., Induction of Molecular Asymmetry by a Remote Chiral Group, Nature 1997, 385, 799-801. c) Clayden A., Lund L., Vallverdú L., Helliwell M., Ultra-remote Stereocontrol by Conformational Communication of Information along a Carbon Chain, Nature 2004, 431, 966-971.

  • For recent reviews concerning trienamine, see: a) Arceo E., Melchiorre P., Extending the Aminocatalytic HOMO-Raising Activation Strategy: Where Is the Limit?, Angew. Chem., Int. Ed. 2012, 51, 5290-5292. b) Kumar I., Ramaraju P., Mir N. A., Asymmetric Trienamine Catalysis: New Opportunities in Amine Catalysis, Org. Biomol. Chem. 2013, 11, 709-716.

  • Jia Z.-J., Jiang H., Li J.-L., Gschwend B., Li Q.-Z., Yin X., Grouleff J., Chen Y.-C., Jørgensen K. A., Trienamines in Asymmetric Organocatalysis: Diels−Alder and Tandem Reactions, J. Am. Chem. Soc. 2011, 133, 5053-5061.

  • a) Lin H., Danishefsky S. J., Gelsemine: A Thought- Provoking Target for Total Synthesis, Angew. Chem., Int. Ed. 2003, 42, 36–51. b) Galliford C. V., Scheidt K. A., Pyrrolidinyl-Spirooxindole Natural Products as Inspirations for the Development of Potential Therapeutic Agents, Angew. Chem., Int. Ed. 2007, 46, 8748-8758. c) Rottmann M. et al., Spiroindolones, a Potent Compound Class for the Treatment of Malaria, Science 2010, 329, 1175-1180.

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