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A series of two-dimensional (2D) arrays of Au-core/Ag-shell nanoparticles with fixed sub-3nm gap distance was obtained on 1cm2 substrates. All 2D arrays resulted in homogeneous and dense monolayers of nanoparticles thanks to our original hybrid deposition method based on self-assembly. Midnanosized gold nanoparticles were used as the core and Ag-shell with different thicknesses were grown to tune...
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