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Mixing enthalpy in LnX 3 –MX liquid systems (M=alkali metal, X=halide) has been analysed. This enthalpy is negative in all systems. The maximum of the absolute value of molar mixing enthalpy depends on the ionic radius of lanthanide(III) and alkali metal cations as well as on the ionic radius of halide anion. The smaller the ionic radius of Ln 3+ , the larger the maximum of the absolute...
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