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The non‐reactive OPLS‐AA force‐field is used to compare direct shock and Hugoniostat simulations of a melt of cis‐1,4‐polybutadiene at different shock velocities and with chain lengths up to 500 monomers. Both methods yield equivalent Hugoniot data with negligible influence of the chain length. However, it is found that the dynamical compression effects induce a time‐dependent anisotropy in the stress...
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